A Brief Summary of the Most Significant Scientific Contributions of Dipankar Home having conceptual, empirical, and practical implications

PREAMBLE

Dipankar Home is the earliest Indian researcher who did his doctoral work on Foundations of Quantum Mechanics in the beginning of 1980s at Presidency College, Kolkata, followed by post-doctoral works in UK (Queen’s University, Belfast; University of Manchester; Birkbeck College, University of London), and subsequently joined Bose Institute, Kolkata as a faculty member in 1987.

He has been steadily contributing to this area over the last four decades resulting in 148 peer-reviewed publications and 2 Research-level books: (a) Conceptual Foundations of Quantum Physics” (Plenum, 1997), and (b)Einstein’s Struggles with Quantum Theory: A Reappraisal” with A. Whitaker (Springer, 2007), with the respective Forewords by 2 Nobel laureates Anthony Leggett and Roger Penrose. Both these books have been appreciatively reviewed in “Physics Today”, the flagship magazine of American Institute of Physics.

During the last few decades, this line of research, earlier not accepted as part of mainstream research pursuits, has remarkably evolved, leading to fundamentally important experiments, and has laid the basis for a frontier area of science, viz. Quantum Information Theory, alongside varied applications in Quantum Communication and Quantum Computation, thereby providing a cornerstone for the 21st Century Quantum Technologies. In fact, while announcing the Nobel Prizes in Physics 2022 for pioneering works in this area, this research area has been acclaimed by the Nobel Committee as a “vibrant and rapidly developing field” which has ushered in the “Second Quantum Revolution.”

Central Themes of the Most Significant Research Works of Home with his Collaborators

(A) Investigations on the interplay between foundational issues of Quantum Mechanics and their experimental realizations, exploring novel features of Quantum Mechanics.

(B) Studies on fundamental topics concerning the interplay between Quantum Foundations, Quantum Information Theory, and Quantum Entanglement enabled applications in secure information transfer/processing protocols.

HIGHLIGHTS

 As has been elaborated in the following, 3 of the proposed experiments by Home and his collaborators have been implemented revealing earlier unexplored quantum features, while 3 other proposed ideas are being pursued for experimental studies. Moreover, Home has contributed to a Theory-Experiment collaboration work which has been experimentally realized, and another such work is underway.

(I) Blending of two fundamental Quantum Features, Indistinguishability and Entanglement, with consequent applications

(a) An earlier unnoticed remarkable property of Entanglement arising from Indistinguishability of any two identical particles was uncovered by us, calling it ‘Duality in Entanglement’ [Physical Review Letters 110, 140404 (2013)].

Using photons, our predicted ‘Duality in Entanglementwas experimentally verified at Tsinghua University, Beijing [New Journal of Physics 16, 083011 (2014)], followed by another photonic experimental study of this property at INRIM, Torino [Physical Review A 91, 062117 (2015)]. An interesting application of this property was also pointed out by others for performing entanglement sorting of photons [Physical Review A 91, 062303 (2015)].

(b) A novel scheme towards harnessing Quantum Indistinguishability for an arbitrarily efficient entanglement generation was formulated by us for any two identical Bosons/Fermions originating from two independent sources [Physical Review Letters 88, 050401 (2002)]. Such a scheme is of considerable significance since Entanglement lies at the core of Quantum Technology of the 21st Century.

While the ideas conceived in this work have been used by others, for example, in the studies concerning Free-electron Quantum Computation [Physical Review Letters 93, 020501 (2004)], the prospect of its experimental realization has now brightened and is being investigated taking advantage of the recent notable technological developments concerning molecular two-particle interferometry and non-absorptive path detectors, the two key ingredients of our scheme.

(II) Formulation of a novel testable scheme for evidencing Quantumness and testing violation of Macrorealism for oscillating objects having large mass

Using the currently available state-of-the-art technology, our work [Physical Review Letters 120, 210402 (2018)] has been successful in formulating a feasible way of testing Quantumness as well as the violation of the basic everyday notion of Macrorealism for optically trapped and harmonically oscillating nano-objects having masses around 106 – 109 amu (about million to billion times heavier than hydrogen atom), much greater than that possible by other methods realised so far. This would, therefore, contribute significantly to the contemporary frontier research enterprise of testing the limits of validity of quantum mechanics in the macroscopic domain. To be more specific, our scheme provides the means for testing the archetypal signature of classicality given by the Leggett-Garg macrorealist inequality (temporal counterpart of Bell-type inequality), currently attracting extensive studies. The implementation of our proposal is being pursued by H. Ulbricht and his group at University of Southampton UK. Apart from the fundamental importance of such an experiment in providing empirical constraints on the various suggested models of wave function collapse beyond standard Quantum Mechanics, the macroscopic quantumness so demonstrated can also have applications like in the area of Quantum Sensing.

(III) Introducing the notion of ‘Single Particle (intraparticle) Entanglement’ and formulating Bell-type inequality for testing Quantum Contextuality, with consequent applications

(a) This work by us was the earliest to come up with the notion of entanglement between two different dynamical variables of a single particle, formulating a general framework for a Bell-type inequality pertaining to such entanglement [Physics Letters A 102, 159 (1984)] based on the notion of Noncontextuality (assuming that the measured value of a dynamical variable does not depend on which other dynamical variable is measured alongside).

(b) We later developed this work by devising an empirically realizable scheme involving specifically path-spin entanglement for a single particle, thereby providing the basis for an experimental demonstration of Quantum Contextuality for the first time by adapting an appropriate form of Bell-type inequality in this context [Physics Letters A 279, 281 (2001)]. The proposed experiment was subsequently performed by the Neutron Interferometric group at Atominstitut, Vienna [Nature 425, 45 (2003)]. This was followed by theoretical and experimental studies by various groups concerning such single particle (intraparticle) entanglement and its applications in quantum information transfer protocols, including our further contributions in this area [Reviewed by S. Azzini et al. in Advanced Quantum Technology, Vol. 3, No. 10 (2020)].

(IV) DNA Molecular scheme for probing the “Schrödinger-Cat” or the Quantum Measurement Problem

DNA molecular analogue of the much-discussed Schrödinger’s Cat example was formulated by us for the first time in the context of the Quantum Measurement Problem in the mesoscopic domain, using the biochemical property of photolyase enzyme attachment to uv-absorbed DNA molecules acting as detectors of uv photons [Physical Review Letters 76, 2836 (1996)]. The way such an example can provide empirically relevant constraints on the wave function collapse models proposed for addressing this central riddle of Quantum Mechanics was analysed by us which played a key role in opening up an earlier uncharted area of study using such systems.

The futuristic significance of this intriguing work was commented upon in “Encyclopaedia Britannica Book of the Year 1996” (edited by G. M. Edwards), pp. 242-243, as well as in the Review article by the Nobel laureate A. J. Leggett, J. Phys. Condens. Matter 14, R415 (2002). In view of the recent advances in studies towards using biomolecular systems for investigating fundamental quantum issues, further development of our original proposal for empirically probing deeper the much-debated aspects of the Quantum Measurement Problem is acquiring more topical significance. 

(V) Revealing an earlier unexplored facet of wave-particle duality of single photons

A testable experiment was proposed by us predicting wave-like optical tunneling as well as particle-like anticoincidences of single photons in the same setup for a double-prism device [Physics Letters A 153, 403 (1991); 168, 95 (1992)], subsequently implemented at the Hamamatsu Photonics Central Research Laboratory, Japan [Physics Letters A 168, 1 (1992)] demonstrating a novel aspect of wave-particle duality. This provided a stimulating twist to the Bohrian principle of wave-particle complementarity by going beyond the usual domain of its application concerning the single particle interference vis-à-vis which-path determination. Conceptual implications of this work had evoked considerable discussions in a number of papers/books. Furthermore, the double-prism device for single photonic experiment developed for this purpose at the Hamamatsu Laboratory, Japan had interesting applications.

(VI) Theory-Experiment Collaboration Work: Single photon based interferometric loophole-free test of the temporal counterpart of Bell inequality, viz. the Leggett-Garg macrorealist inequality

This work developed by providing the required theoretical inputs, in collaboration with U. Sinha’s experimental quantum optics group at Raman Research Institute, Bangalore, resulted in an unambiguous demonstration of the empirical violation of the Leggett-Garg inequality, thereby decisively repudiating the notion of realism for single photons, by closing all the relevant loopholes (including the most important ones, detection efficiency and clumsiness loopholes) for the first time by using appropriately devised strategies [Physical Review X Quantum 3, 010307 (2022)].

Thus, this experimental platform provides a powerful means for certifying inherent nonclassicality of single photons which can be reliably and efficiently harnessed towards Quantum Communication based applications for which the single photon is a ubiquitous workhorse.

(VII) Exploring novel uses and fundamental implications of the temporal counterpart of Bell inequality, viz. the Leggett-Garg macrorealist inequality

(a) In the case of arbitrarily large spins, even under the coarsening of measurement times, coupled with the coarsening of measurement outcomes, the persistence of quantum mechanical violation of the Leggett-Garg inequality implying incompatibility with the notion of macrorealism was shown in our work for the first time [Physical Review A 94, 052110 (2016); Physical Review A 100, 042114 (2019)]. This striking feature revealed that classicality for large spin does not emerge from quantum mechanics, whatever be the form and degree of ‘unsharpness’ or coarse graining of the measurements outcomes. Such finding has fundamental implications concerning the much debated issue of the Classical Limit of Quantum Mechanics.

(b) Our work [Physical Review A 88, 022115 (2013)] was the first to probe implications of the quantum mechanical violation of the Leggett-Garg inequality in the context of weak interaction induced two state oscillations of neutral kaons and neutrinos. A remarkable result was obtained that this violation for the kaon oscillation is enhanced due to CP noninvariance, while, for the neutrino oscillation, such violation is sensitively dependent on the value of the mixing parameter. This work opened up a potentially rich area, inspiring other studies, including an important experiment [Physical Review Letters 117, 050402 (2016)] which demonstrated quantum mechanically predicted violation of the Leggett-Garg inequality for neutrino oscillation over a length scale of nearly 700 km. Further studies are underway, including trying to unravel the deeper ramifications of this experiment, in conjunction with the implications of our earlier initiating work on this topic.

(VIII) Generalising Wigner’s approach for detecting Multipartite Nonlocality

(a) Distinct from Bell’s approach, Wigner had suggested an elegant formulation of local realist inequality for showing quantum nonlocality. However, Wigner’s original scheme was restricted to only bipartite maximally entangled states, and hence was largely ignored. Our work [Physical Review A 91, 012102 (2015)] was the first to successfully generalise Wigner’s approach towards detecting nonlocality of an arbitrary multipartite entangled state by deriving appropriate local realist multipartite inequalities. Thus, this work opened up an earlier unexplored direction for studying multipartite nonlocality, a topic which is of much contemporary interest.

(b) Recently, we followed up our preceding work by showing that Wigner’s approach can be further developed by deriving a suitable set of local realist multipartite inequalities having the following important feature. Their quantum mechanical violation can not only rigorously certify multipartite nonlocality for any multipartite entanglement by considering all its different bipartitions, but can also enable detecting whether there is any particular bipartition of the multipartite system which is nonlocally correlated for cases where not all different bipartitions are nonlocally correlated [Physical Review A 106, 062203 (2022)]. This additional feature provides our formulated extension of Wigner’s scheme a significant advantage compared to the other standard multipartite nonlocality detection scheme based on using the Svetlichny inequality. The efficacy of our scheme has been comprehensively illustrated for the tripartite and quadripartite states.

(IX) Formulating novel approaches for studying Quantification and Uses of Quantum Entanglement as Resource

 (a) Using Pearson Correlators for Quantifying Higher Dimensional Entanglement

In view of considerable advantages provided by the high dimensional entangled states for ensuring efficient and robust applications in Quantum Communication, the quantification of high dimensional entanglement is of much topical importance for enabling judicious assessment of the usefulness of a given entangled state for its efficient applications.  In this context, our work [Physical Review A 101, 022112 (2020)] initiated a novel direction of study in terms of the empirically measurable statistical correlator known as the Pearson Correlator, which we analytically related with a suitable entanglement measure like Negativity for a range of bipartite pure and mixed qutrit states using only a pair of complementary observables in each wing of the bipartite system. This approach, therefore, opens up unique empirical means for exactly quantifying such higher dimensional entanglement measure. Extension of this scheme for a wider class of high dimensional bipartite entangled states using Pearson Correlator and other statistical correlators like Mutual Predictability and Mutual Information is a promising area of research with multifold applications in Quantum Information and Quantum Communication, and our research work along this direction is currently in progress.

 

(b) Appropriate Quantification of the effectiveness of any Resource State for implementing Remote State Preparation

In this work [Physical Review A 98, 062320 (2018)] we show that an appropriate measure of simultaneous correlations in mutually unbiased bases can serve as a powerful quantifier of the usefulness of a resource state for Remote State Preparation (RSP) based on bipartite entangled as well as separable states, even using zero-discord states. Given the importance of RSP as a key Quantum Information Processing task, further works harnessing the potentiality of this novel approach should be of considerable significance.

(c) Identifying the appropriate Quantitative Measure of effectiveness of any Resource State for Quantum Steering

Besides its fundamental implications, the phenomenon of Quantum Steering has wide-ranging useful Quantum Information Processing applications. However, an outstanding issue underlying such applications is the question concerning what aspect of bipartite Quantum Correlation can serve as the appropriate quantitative resource for Quantum Steering. This has, surprisingly, remained unaddressed. It is in this work [Physical Review A 98, 042306 (2018)] we have resolved this issue by analytically relating an appropriate measure of simultaneous correlations in mutually unbiased bases to the standard measure of Quantum Steering used for two-qubit states so that a higher value of the measure of such correlations implies a higher degree of Quantum Steering. This scheme, thus, opens up a promising line of studies towards further developing this approach and exploring its potential applications by harnessing Quantum Steering in areas like Quantum Communication.

ONGOING AND PLANNED RESEARCH PROGRAMMES WITH VARIOUS COLLABORATORS

A. Formulating and Developing novel ideas for testing Macroscopic Quantumness, with possible applications in Quantum Technologies

(i) In the context of one of the most topically important challenging enterprises of contemporary physics seeking to test the limits of applicability of quantum mechanics, a cutting-edge scheme is being formulated capable of demonstrating mass-independent quantumness of a harmonically oscillating levitated large mass nano-object. This is realisable with the state-of-the-art technology, entailing potential rich applications in areas like Quantum Sensing, apart from having significant implications in empirically constraining various wave function collapse models proposed for Quantum Measurements. Importantly, our proposed scheme offers the tantalizing prospect of scaling up the test of quantumness, all the way to arbitrarily massive linear oscillators, with the flexibility of choosing the relevant parameters within the accuracy of standard quantum limit. A preliminary version of this work is in the arXiv:2211.10318, currently being developed further, in collaboration with the relevant experimental group at University of Southampton, UK.

(ii) Using the novel idea of massive spatial qubits, we are formulating a testable proposal for evidencing macro-nonclassicality as well as Casimir interaction induced entanglement between two neutral nano-objects of mass about billion – trillion times more than that of hydrogen atom. This would enable testing for the first time quantumness of Casimir interaction persisting in the macroscopic domain. A preliminary version of this work is in the arXiv:2106.11906, currently being developed further.

(iii) Testing the quantum nature of gravity is yet another fundamentally important open question in the frontiers of contemporary physics. To this end, we are formulating a scheme in detail so that we can apply our idea of massive spatial qubits by encoding qubit in the spatial degree of freedom of a freely propagating massive object towards experimentally detecting the gravitational interaction induced entanglement generated between two spatial superpositions of states of massive objects. This would constitute a novel way of evidencing the quantumness of gravity for massive objects with far-reaching fundamental implications as well as having potentialities for applications in Quantum Sensing. A preliminary version of this work is in the arXiv:2211.03661, currently being developed further.

(iv) Currently investigating critically the basis of Larmor precession and seeking to analyse how the spatial-spin coupling in a single spin ½ particle wavefunction while traversing a region of confined uniform magnetic field can induce deviation from Larmor precession in such a way that persists for significantly large masses and can have applications for Quantum Sensing.

B. On Quantum enabled schemes for Device-independent Genuine Random Number Generators

 (a) In view of the crucial role played by Genuine Random Numbers for guaranteeing secure encryption of information in various protocols of Quantum Communication (including Cryptography), even while using untrustworthy devices, the study of schemes for generating device-independent Genuine Random Numbers (secure against device-tampering and eavesdropping) is of much topical importance. In this context, a comprehensive research programme is being pursued for certifying and quantifying device-independent Genuine Random Numbers based on harnessing Quantum Nonlocality through the use of Hardy and Cabello-Liang type nonlocality arguments based on two-qubit entangled states. This also involves the study of quantitative relationship between Nonlocality and Randomness which seems to reveal features which were not seen earlier by using the Bell inequality based nonlocality argument for analysing this issue.

(b) While all the studied scheme to date for generating device-independent Genuine Random Numbers have been based on Nonlocality arising from Quantum Entanglement, we are currently trying to formulate an alternative approach for this purpose without relying on entangled systems as resource. Instead, we are making use of the quantumness of an individual system evidenced through the quantum violation of the temporal counterpart of the Bell inequality (known as the Leggett-Garg inequality). We have already worked out how to certify device-independent Genuineness of Random Numbers using the Leggett-Garg inequality (LGI) pertaining to the time evolution of a single system. Currently, we are in the midst of rigorously developing the procedure for suitably quantifying such certified randomness. Once such quantification scheme is fully worked out, the present work will provide the basis for a new generation of LGI based Genuine Random Number Generators using single systems. This will be practically advantageous compared to the Bell inequality based ones because the latter require entangled systems having sufficient spatial separation between them, and such an entanglement across distance needs to be preserved over sufficient time against decoherence effects, which is experimentally challenging to ensure. The next key step in this Research Programme will be to analyse the experimental implementability of our proposed scheme. Towards this goal, we have already initiated interactions with the relevant experimental group (at Raman Research Institute, Bangalore) using single photons.

C. On Exploring Applications of Intraparticle Quantum Entanglement in Quantum Communication

 

Developing further our earlier works introducing the idea of entanglement between two different properties of a single particle (called intraparticle entanglement) and subsequently formulating scheme for experimentally testing implications of this form of entanglement (Physics Letters A 102, 159 (1984); 279, 281 (2001)) which have inspired a range of sequel works by various groups including ours (reviewed in Advanced Quantum Technology, Vol. 3, No. 10 (2020), investigations are now being launched for devising practically viable uses of such entanglement between different dynamical variables of a single particle in the context of various information transfer/processing protocols in Quantum Communication, including in Quantum Cryptography. The advantages gained in using such entanglement will be compared with that of the interparticle entanglement based protocols. To this end, an initiating work trying to theoretically formulate a suitable variant of the dense coding protocol is in progress, apart from pursuing interactions with the relevant photonic experimental group at Raman Research Institute, Bangalore for probing the implementability of a number of ingenious ideas in this context.

D. On Quantifying High Dimensional Quantum Entangled States for facilitating their effective applications

 This line of studies has considerable significance in exactly quantifying arbitrary dimensional bipartite entangled states, thereby enabling effective optimization of their possible uses in various applications based on information transfer/processing protocols. Developing further our earlier work [Phys. Rev. A 101, 022112 (2020)] which had initiated the study of a novel method for determining bipartite higher dimensional entanglement measures using empirically measurable statistical correlators, a comprehensive study is in progress for analytically relating an entanglement measure like Negativity with the observable statistical correlators like Pearson Correlator, Mutual Predictability, and Mutual Information for a range of empirically relevant bipartite arbitrary dimensional mixed entangled states, importantly using only a pair of complementary observables in each wing of the bipartite system. Extension of this study for tripartite arbitrary dimensional entangled states is also in progress.

E. Unravelling aspects of Quantum Nonlocality in the pursuit of fresh insights and newer applications

 (i) An investigation is underway from an earlier unexplored perspective trying to probing the nature of Nonlocality within Quantum Mechanics by invoking what has been called Local Friendliness inequality in this context for the first time by using a modified Einstein-Podosky-Rosen-Bohm setup. This approach, apart from its wider conceptual implications, has the potentiality to usefully complement the standard approach based on Bell-type inequalities towards different forms of applications of Quantum Nonlocality in Quantum Communication.

(ii) The nonlocal feature of Quantum Teleportation is being probed by formulating preparation noncontextuality based local realist inequality for the first time, seeking to provide deeper understanding of the way nonlocality occurs in Quantum Teleportation. The way the quantum feature of preparation contextuality is being used in this work for showing nonlocality is strikingly distinct from the standard Bell-type inequality based nonlocality arguments, and can have wider ramifications. In particular, the insights thus obtained can provide clues for harnessing Quantum Nonlocality more efficiently towards implementing various protocols of Quantum Communication.

 F. Demonstration of the Quantum Cheshire Cat effect

An important Theory-Experiment collaboration work is nearing completion with theoretical inputs and the expt. being performed at Raman Research Institute, Bangalore by Urbasi Sinha’s group. This experiment seeks to realise for the first time joint detection of spatially separated two properties like spatial and polarization degrees of freedom of a single photon in the two respective arms of an interferometer in each run of the experiment. This is being achieved by implementing non-destructive and minimally-disturbing interactions in both arms of the interferometer, with each such interaction coupling a suitable particle property to a pointer while maintaining the superposition of single photon states corresponding to propagation along the different arms of the interferometer. Such an experiment would constitute an unambiguous demonstration of what has been called the Quantum Cheshire Cat effect entailing joint detection of different properties of an individual particle in the respective two arms of the interferometer. Such an intriguing effect would have far-reaching conceptual implications and potentiality for interesting applications in the context of Quantum Sensing and Information transfer/processing protocols which should be worth investigating in a sequel work. Preliminary experimental results of this work have been reported in the arXiv:2201.11425.

G. Exploring implications of the Quantum Zeno Effect towards its various applications

Inhibition of the time evolution of a quantum system due to repeated frequent measurements, even if these measurements are classically nondisturbing, is known as the Quantum Zeno effect (QZE). This striking Quantum Effect has deep-seated conceptual ramifications which have been much discussed in the relevant literature since it was first pointed out in 1977 and subsequently experimentally first demonstrated in 1990. However, surprisingly, the study of QZE in the context of Quantum Entanglement has yet remined unexplored and possible applications of QZE have not been much discussed. It is this gap we seek to fill in through the following two Research Programmes by taking clues from our earlier extensive studies on QZE in the 1980s and 90s, culminating in our widely cited Review article on QZE [Annals of Physics 258, 237 (1997)]:

(i) Since the preservation of Quantum Entanglement in the presence of any decohering environment is an important requirement in any application of Entanglement, the inhibition of the time evolution of an entangled state due to QZE in the presence of a decohering medium can play a key useful role in this context. We propose to systematically study in detail to show comprehensively the way QZE can be effective in contributing to preserve entanglement in the presence of various physically relevant damping channels like amplitude/phase damping channels by inhibiting the decay of entanglement in these damping channels.

(ii) Another tantalising prospective application of QZE is in the context of the cutting-edge research area of testing Macroscopic Quantumness and harnessing it for applications in futuristic Quantum Technologies. To this end, we have started working on a Research Programme for making effective use of QZE in a way that can enable showing empirically appreciable amplification of the effect of Macroscopic Quantumness that can be evidenced through the much enhanced violation of the Leggett-Garg inequality whose violation is an archetypal signature of intrinsic Quantumness.

 

Current Principal Collaborators

S. Bose (University College London, UK); U. Sinha (Raman Research Institute, Bangalore); P. Panigrahi (IISER, Kolkata); A. S. Majumdar (S. N. Bose National Centre for Basic Sciences, Kolkata); A. Matzkin (CNRS, Univ. de Cergy, France); H. Ulbricht (University of Southampton, UK); A. Banerjee (IISER, Pune); A. Majumdar (University of Groningen, Netherlands); D. Saha (IISER, Thiruvananthapuram); S. Das (LMU Munich, Germany); S. Jain (IISER, Pune).

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